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Fluorescence lifetime measurements in a polymer chain are modeled using a memory function expansion, computer simulations, and simple scaling arguments. Unless the quenching rate is localized and infi...
Single molecule experiments reveal intriguing phenomenon in chemical and biological systems.Several indicators of complex dynamics, including ‘‘intensity’’ correlations, ‘‘event’’ correlations,and cha...
The configuration-controlled regime and the diffusion-controlled regime of conformation-modulated fluorescence emission are systematically studied for Markovian and non-Markovian dynamics of the react...
Stationary and nonstationary multilevel models are formulated to analyze ultrafast multiphoton processes with emphasis on electronic and nuclear coherence of a near-resonant intermediate state. By ide...
The Zewail–Bersohn model@Ber. Bunsenges. Phys. Chem.92, 373 ~1988!# of pump–probe experiments is generalized to nonstationary wave packets and more realistic forms of probe pulses. The analysis illust...

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